From ff709ebe19ae5bfba3c6e28d913bca3e234d7d74 Mon Sep 17 00:00:00 2001 From: Kostas Vilkelis <kostasvilkelis@gmail.com> Date: Mon, 6 May 2024 13:15:09 +0200 Subject: [PATCH] finish writing eqs;proceed to numerical algo description --- docs/source/mf_notes.md | 75 +++++++++++++++++++++++++++++------------ 1 file changed, 53 insertions(+), 22 deletions(-) diff --git a/docs/source/mf_notes.md b/docs/source/mf_notes.md index 3b57aa1..f486ad3 100644 --- a/docs/source/mf_notes.md +++ b/docs/source/mf_notes.md @@ -1,58 +1,89 @@ # Algorithm overview -## Interacting problems +## Derivation of the mean-field Hamiltonian + +### Interacting problems In physics, one often encounters problems where a system of multiple particles interact with each other. In this package, we consider a general electronic system with density-density interparticle interaction: :::{math} :label: hamiltonian -\hat{H} = \hat{H_0} + \hat{V} = \sum_{ij} h_{ij} c^\dagger_{i} c_{j} + \frac{1}{2} \sum_{ij} v_{ij} c_i^\dagger c_j^\dagger c_j c_i +\hat{H} = \hat{H^0} + \hat{V} = \sum_{ij} h_{ij} c^\dagger_{i} c_{j} + \frac{1}{2} \sum_{ij} v_{ij} c_i^\dagger c_j^\dagger c_j c_i ::: where $c_i^\dagger$ and $c_i$ are creation and annihilation operators respectively for fermion in state $i$. -The first term $\hat{H}_0$ is the non-interacting Hamiltonian which by itself is straightforward to solve in a single-particle basis by direct diagonalizations made easy through packages such as `kwant`. +The first term $\hat{H^0}$ is the non-interacting Hamiltonian which by itself is straightforward to solve in a single-particle basis by direct diagonalizations made easy through packages such as `kwant`. The second term $\hat{V}$ is density-density interaction term between two particles, for example Coulomb interaction. In order to solve the interacting problem exactly, one needs to diagonalize the full Hamiltonian $\hat{H}$ in the many-particle basis which grows exponentially with the number of particles. Such a task is often infeasible for large systems and one needs to resort to approximations. -## Mean-field Hamiltonian +### Mean-field approximaton The first-order perturbative approximation to the interacting Hamiltonian is the Hartree-Fock approximation also known as the mean-field approximation. The mean-field approximates the quartic term $\hat{V}$ in {eq}`hamiltonian` as a sum of bilinear terms weighted by the expectation values the remaining operators: - -$$ +:::{math} +:label: mf_approx \hat{V} \approx \hat{V}^{\text{MF}} \equiv \sum_{ij} v_{ij} \left[ \braket{c_i^\dagger c_i} c_j^\dagger c_j - \braket{c_i^\dagger c_j} c_j^\dagger c_i \right] -$$ - +::: we neglect the superconducting pairing and constant offset terms. -The expectation value terms $\langle c_i^\dagger c_j \rangle$ are due to the ground-state density matrix: - -$$ -\rho_{ij} \equiv \langle c_i^\dagger c_j \rangle, -$$ - -and therefore act as an effective field acting on the system. +The expectation value terms $\langle c_i^\dagger c_j \rangle$ are due to the ground-state density matrix and therefore act as an effective field acting on the system. +The ground-state density matrix reads: +:::{math} +:label: density +\rho_{ij} \equiv \braket{c_i^\dagger c_j } = \text{Tr}\left(e^{-\beta \left(\hat{H^0} + \hat{V}^{\text{MF}} - \mu \hat{N} \right)} c_i^\dagger c_j\right), +::: +where $\beta = 1/ (k_B T)$ is the inverse temperature, $\mu$ is the chemical potential, and $\hat{N} = \sum_i c_i^\dagger c_i$ is the number operator. -<!-- :::{admonition} Derivation of the mean-field Hamiltonian with Wicks theorem +:::{admonition} Derivation of the mean-field Hamiltonian with Wicks theorem :class: dropdown info ```{include} mf_details.md ``` -::: --> +::: -### Tight-binding grid +### Finite tight-binding grid -To simplify the mean-field Hamiltonian, we assume a normalised orthogonal tight-binding grid defined by the single-particle basis states: +To simplify the mean-field Hamiltonian, we assume a finite, normalised orthogonal tight-binding grid defined by the single-particle basis states: $$ \ket{n} = c^\dagger_n\ket{\text{vac}} $$ where $\ket{\text{vac}}$ is the vacuum state. -We project our mean-field interaction onto the tight-binding grid: +We project our mean-field interaction in {eq}`mf_approx` onto the tight-binding grid: + +:::{math} +:label: mf_finite +V^\text{MF}_{nm} = \braket{n | \hat{V}^{\text{MF}} | m} = \sum_{i} \rho_{ii} v_{in} \delta_{nm} - \rho_{mn} v_{mn}, +::: +where $\delta_{nm}$ is the Kronecker delta function. + +### Infinite tight-binding grid + +In the limit of a translationally invariant system, the index $n$ that labels the basis states partitions into two independent variables: the unit cell internal degrees of freedom (spin, orbital, sublattice, etc.) and the position of the unit cell $R_n$: $$ -V^\text{MF}_{nm} = \langle n | \hat{V}^{\text{MF}} | m \rangle = \sum_{i} \rho_{ii} v_{in} \delta_{nm} - \rho_{mn} v_{mn}, +n \to n, R_n. $$ -where $\delta_{nm}$ is the Kronecker delta function. + +Because of the translationaly invariance, the physical properties of the system are independent of the absolute unit cell position $R_n$ and rather depend on the relative position between the two unit cells $R_{nm} = R_n - R_m$: + +$$ +\rho_{mn} \to \rho_{mn}(R_{mn}). +$$ + +That allows us to re-write the mean-field interaction in {eq}`mf_finite` as: + +:::{math} +:label: mf_infinite +V^\text{MF}_{nm} (R) = \sum_{i} \rho_{ii} (0) v_{in} (0) \delta_{nm} \delta(R) - \rho_{mn}(R) v_{mn}(R), +::: + +where now indices $i, n, m$ label the internal degrees of freedom of the unit cell and $R$ is the relative position between the two unit cells in terms of the lattice vectors. + +## Numerical solution of the mean-field Hamiltonian + +In order to calculate the mean-field interaction in {eq}`mf_infinite`, we require the ground-state density matrix $\rho_{mn}(R)$. +However, the density matrix in {eq}`density` is a functional of the mean-field interaction $\hat{V}^{\text{MF}}$ itself. +Therefore, -- GitLab